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《武汉工程大学学报》[ISSN:1674-2869/CN:42-1779/TQ]

卷:: 45
期数:: 2023年04期

页码:: 364-377

栏目:: 综述

出版日期:: 2023-08-31

文章信息/Info

Title:: Research Progress in MXene-Based Electrocatalysts for
Hydrogen Production from Water Electrolysis

文章编号:: 1674 - 2869（2023）04 - 0364 - 14

作者:: 王东¹; 杨圣雄²; 肖健³; 王贵生⁴; 肖军武²; 孙义民^*1; 1. 等离子体化学与新材料湖北省重点实验室（武汉工程大学），湖北武汉 430205；
2. 华中科技大学化学与化工学院，能量转换与储存材料化学教育部重点实验室，湖北武汉 430074；
3. 武汉工程大学化工与制药学院，湖北武汉 430205；
4. 中国石化胜利油田安全环保质量管理部能源环境办公室，山东东营 257001

Author(s):: WANG Dong¹; YANG Shengxiong²; XIAO Jian³; WANG Guisheng⁴; XIAO Junwu²; SUN Yimin^*1; 1. Hubei Key Laboratory of Plasma Chemistry and Advanced Materials（Wuhan Institute of Technology），Wuhan 430205，China；
2. Key Laboratory of Material Chemistry for Energy Conversion and Storage，Ministry of Education，School of Chemistry and Chemical Engineering，Huazhong University of Science and Technology，Wuhan 430074，China；
3. School of Chemical Engineering and Pharmacy，Wuhan Institute of Technology，Wuhan 430205，China；

关键词:: MXene; 电解水; 析氢反应; 析氧反应

Keywords:: MXene; water electrolysis; hydrogen evolution reaction; oxygen evolution reaction

分类号:: TQ127

DOI:: 10.19843/j.cnki.CN42-1779/TQ.202209001

文献标志码:: A

摘要:: MXene因其优异的物理和化学特性，在电解水领域极具应用潜力。对电解水阴极析氢反应和阳极析氧反应中使用的MXene基材料进行了归纳和总结，通过分析可知，非金属元素掺杂、单/多金属元素负载以及结构设计等策略，已成为提高MXene电催化性能强有力的手段。此外，针对MXene在构建电解水催化剂中存在的缺点，诸如种类有限、表面基团不可控、易氧化、污染性等，提出了开发MXene新种类、寻找新型合成方法、与纳米材料复合增强稳定性以及采用无氟环保刻蚀剂等应对策略。

Abstract:: MXene possesses great potential for water electrolysis application due to its excellent physical and chemical properties. In this paper，MXene-based composites used in hydrogen evolution reaction and anode oxygen evolution reaction were summarized. Through the analysis，we can see that non-metal element doping，single/multi-metal element loading and the structure design have become powerful means to improve the performance of MXenes electrocatalysis. Aiming at the shortcomings of MXene in the construction of electrolytic water catalyst，such as limited species，uncontrollable surface groups，easy oxidation and pollution， we propose the corresponding coping strategies，i.e. developing new types of MXene，searching for new synthesis methods，compositing with nano-materials to enhance stability，and using fluorine-free environment-friendly etchants， to solve those problems.

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备注/Memo

备注/Memo:: 收稿日期：2022-09-02
基金项目：国家自然科学基金（51504168）；湖北省教育厅科学研究计划指导性项目（B2021075）；武汉工程大学第十三届研究生教育创新基金（CX2021152）
作者简介：王东，硕士研究生。E-mail：[email protected]
*通讯作者：孙义民，博士，副教授。E-mail：[email protected]
引文格式：王东，杨圣雄，肖健，等. 用于电解水制氢的MXene基电催化剂的研究进展［J］. 武汉工程大学学报，2023，45（4）：364-377，412.

更新日期/Last Update: 2023-08-31

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